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Compounds

COMPOUND NPA003891

STRUCTURE
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PROPERTIES
NPAID NPA003891
CLUSTER ID 2095
NODE ID 1677
NAME Berkelic acid
FORMULA C29H40O9
MOLECULAR WEIGHT (Da) 532.6300
ACCURATE MASS (Da) 532.2672
ORIGIN ORGANISM TYPE Fungus
ORIGIN GENUS Penicillium
ORIGIN SPECIES sp.
InChIKey KUPCHRRTAPZASB-FZIMWOAESA-N
InChI InChI=1S/C29H40O9/c1-6-8-9-10-19-11-17-12-20(30)24(26(32)33)25-23(17)21(37-19)14-29(38-25)16(3)18(15-36-29)13-22(31)28(4,7-2)27(34)35-5/h12,16,18-19,21,30H,6-11,13-15H2,1-5H3,(H,32,33)/t16-,18+,19+,21-,28-,29-/m0/s1
SMILES CCCCC[C@@H]1CC2=CC(O)=C(C(=O)O)C3=C2[C@H](C[C@]2(OC[C@@H](CC(=O)[C@](C)(CC)C(=O)OC)[C@@H]2C)O3)O1
ORIGINAL ISOLATION REFERENCE
CITATION Stierle, Andrea A.; Stierle, Donald B.; Kelly, Kal Berkelic Acid, A Novel Spiroketal with Selective Anticancer Activity from an Acid Mine Waste Fungal Extremophile Journal of Organic Chemistry 2006 71 (14) 5357-5360.
DOI 10.1021/jo060018d PMID 16808526
ORIGINAL ISOLATION TAXONOMY
RANK NAME DB LINK NCBI
Domain Eukarya - 2759
Kingdom Fungi MycoBank 4751
Phylum Ascomycota MycoBank 4890
Class Eurotiomycetes MycoBank 147545
Order Eurotiales MycoBank 5042
Family Aspergillaceae MycoBank 1131492
Genus Penicillium MycoBank 5073
SYNTHESES
CITATION 1 Bender CF; Yoshimoto FK; Paradise CL; De Brabander JK A concise synthesis of berkelic acid inspired by combining the natural products spicifernin and pulvilloric acid. Journal of the American Chemical Society 2009 131 (32) 11350-2. DOI: 10.1021/ja905387r PMID: 19722648
CITATION 2 Snaddon TN; Buchgraber P; Schulthoff S; Wirtz C; Mynott R; Fürstner A Total synthesis of berkelic acid. Chemistry - A European Journal 2010 16 (40) 12133-40. DOI: 10.1002/chem.201001133 PMID: 20853286
CITATION 3 Fañanás FJ; Mendoza A; Arto T; Temelli B; Rodríguez F Scalable total synthesis of (-)-berkelic acid by using a protecting-group-free strategy. Angewandte Chemie International Edition 2012 51 (20) 4930-3. DOI: 10.1002/anie.201109076 PMID: 22488814
CITATION 4 Bender CF; Paradise CL; Lynch VM; Yoshimoto FK; De Brabander JK A biosynthetically inspired synthesis of (-)-berkelic acid and analogs. Tetrahedron 2018 74 (9) 909-919. DOI: 10.1016/j.tet.2018.01.021 PMID: 29867257
REVISIONS
VERSION SMILES CITATION
Original Isolation CCCCC[C@@H]1CC2=CC(=C(C3=C2C(O1)C[C@]4(O3)[C@@H]([C@H](CO4)CC(=O)C(C)(CC)C(=O)OC)C)C(=O)O)O Stierle, Andrea A.; Stierle, Donald B.; Kelly, Kal Berkelic Acid, A Novel Spiroketal with Selective Anticancer Activity from an Acid Mine Waste Fungal Extremophile Journal of Organic Chemistry 2006 71 (14) 5357-5360. DOI: 10.1021/jo060018d PMID: 16808526
2 CCCCC[C@@H]1CC2=CC(O)=C(C(=O)O)C3=C2[C@H](C[C@]2(OC[C@@H](CC(=O)[C@](C)(CC)C(=O)OC)[C@@H]2C)O3)O1 Wu, Xiaoxing; Zhou, Jingye; Snider, Barry B Introduction of the (-)-berkelic acid side chain and assignment of the C-22 stereochemistry. Journal of Organic Chemistry 2009 74 (16) 6245-52. DOI: 10.1021/jo901221a PMID: 19630376
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